Was the cash for the bank's use? If so, a CTR is not required for another financial institution.
A CTR is required unless you exempt them, which is very easy now that a DOEP is not required for them. While the initial DOEP and annual review are not a requirement, a bank still needs to take the same steps to verify the customer's initial eligibility for the exemption and document it.
If you decide not to exempt them, the CTR should be completed with the bank's information in section A and the manager's information in section B of Part I.